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Encapsulation Technologies -- Eliminating Airborne Contamination

Criticality Calculations
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5.0 DISCUSSION OF CONTINGENCIES
There are two criticality scenarios associated with the use of Capture Coating & InstaCote material to remove surface contamination from a glovebox and ancillary equipment, which can be shown to meet the requirements of the double contingency principle.

Scenario #1:  Either 520 grams of Pu in a compact or spherical homogeneous aqueous mixture which is optimally moderated and fully reflected by water (indirectly via Reference 2), or 270 grams of Pu in a compact or spherical homogeneous mixture of Capture Coating & InstaCote (i.e., InstaCote) material which is optimally moderated and fully reflected by water.

Upset Condition
1 270 grams of fissile material accumulate in the Capture Coating & InstaCote material
Barrier
1.1. Assay scans will be performed prior to the use of stripcoat within the glovebox. Assay scans must show that at the upper 95% confidence level for the measurement, there is less than 200 grams of fissile material in the glovebox if the entire box is to have the stripcoat applied and removed.
1.2. If Assay scans indicate greater than 200 grams of fissile material are present inside a glovebox, then only a section of stripcoat, which would contain a maximum of 200 grams fissile material, may be removed at a time. The allowable area of stripcoat can be determined from areal density assay data.
2 Material forming an optimally moderated, compact shape
2.1. Controls restrict geometric volume to 4 liters or less. Restriction to 4 liters or less in volume precludes the formation of the necessary volume for criticality. A Pu mass of 520 grams will be critical if it is homogeneously mixed with water in an approximately 17-liter spherical shape (12.5 inch diameter) and fully reflected with water. A Pu-239 mass of 270 grams will be critical if it is homogeneously mixed with InstaCote material in an approximately 6-liter spherical shape (8.9-inch diameter) and fully reflected with water, but realistic isotopic mixtures of RFETS plutonium would still be subcritical by greater than 2 percent.

Scenario #2: Two 4-liter containers of 1.629-g/cc Capture Coating & InstaCote containing 200 gram of fissile material (specifically plutonium).

Upset Condition
1 Two 200-gram, 4-liter containers of 1.629-g/cc Capture Coating & InstaCote are collected without the first of the two containers being removed from the area before the second is filled.
Barrier
1.1. Administrative procedures and posted controls require removal of 200 grams of accumulated stripcoat prior to generating/accumulating a second batch.
1.2.

Controls restrict individual geometric volumes to 4 liters or less. Restriction to 4 liters or less in volume precludes the formation of the necessary volume for criticality in one container. A Pu mass of 520 grams homogeneously mixed with water in an approximately 17-liter spherical shape (12.5 inch diameter) and fully reflected with water will be critical. A Pu-239 mass of 270 grams homogeneously mixed with InstaCote material in an approximately 6-liter spherical shape (8.9-inch diameter) and fully reflected with water will be critical, also, but realistic isotopic mixtures of RFETS plutonium would still be subcritical by greater than 2 percent. Two 4-liter cylindrical volumes (adjacent to each other and without the presence of a container) each having their height equal to their diameter and each containing a Pu-239 mass of 200 grams homogeneously mixed with InstaCote material will be slightly supercritical (see Table 1, Case E); however, this scenario is unrealistic--the same two volumes having 200 grams of the most reactive RFETS plutonium isotopic mixture, i.e., the RFRAG mixture, would be subcritical by approximately 4 percent.

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